Experimental investigation of fission gas release from spent nuclear fuels under conditions expected in a deep geological repository
Tobias König
CORRESPONDING AUTHOR
Institute for Nuclear Waste
Disposal, Karlsruhe Institute of Technology, P.O. Box 3640, 76021 Karlsruhe, Germany
Elke Bohnert
Institute for Nuclear Waste
Disposal, Karlsruhe Institute of Technology, P.O. Box 3640, 76021 Karlsruhe, Germany
Ernesto González-Robles
Gestión de Proyectos Internacionales, Institut d'Investigació Sanitària Illes Balears (IdISBa), 07120 Palma, Spain
Michel Herm
Institute for Nuclear Waste
Disposal, Karlsruhe Institute of Technology, P.O. Box 3640, 76021 Karlsruhe, Germany
Luis Iglesias-Pérez
Institute for Nuclear Waste
Disposal, Karlsruhe Institute of Technology, P.O. Box 3640, 76021 Karlsruhe, Germany
Volker Metz
Institute for Nuclear Waste
Disposal, Karlsruhe Institute of Technology, P.O. Box 3640, 76021 Karlsruhe, Germany
Arndt Walschburger
Institute for Nuclear Waste
Disposal, Karlsruhe Institute of Technology, P.O. Box 3640, 76021 Karlsruhe, Germany
Horst Geckeis
Institute for Nuclear Waste
Disposal, Karlsruhe Institute of Technology, P.O. Box 3640, 76021 Karlsruhe, Germany
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Our contribution focuses on the release of fission gases during the dissolution process of two different types of spent nuclear fuel, i.e. UOX and (U, Pu)OX mixed-oxide fuels, in order to identify and quantify the role of fission gas release rates as an indicator of radionuclide source terms. Within our work, it is shown that, independent of the type of spent nuclear fuel, a comparable, fast initial release of fission gases is evident in all experiments.
Our contribution focuses on the release of fission gases during the dissolution process of two...