Spectroscopic and chemical investigations on volatile fission and activation products within the fuel-cladding interface of irradiated pressurised water reactor fuel rod segments
Tobias König
CORRESPONDING AUTHOR
Karlsruhe Institute of Technology (KIT), Institute for Nuclear Waste Disposal, P.O. Box 3640, 76021 Karlsruhe, Germany
Ron Dagan
Karlsruhe Institute of Technology (KIT), Institute for Nuclear Waste Disposal, P.O. Box 3640, 76021 Karlsruhe, Germany
Kathy Dardenne
Karlsruhe Institute of Technology (KIT), Institute for Nuclear Waste Disposal, P.O. Box 3640, 76021 Karlsruhe, Germany
Michel Herm
Karlsruhe Institute of Technology (KIT), Institute for Nuclear Waste Disposal, P.O. Box 3640, 76021 Karlsruhe, Germany
Volker Metz
Karlsruhe Institute of Technology (KIT), Institute for Nuclear Waste Disposal, P.O. Box 3640, 76021 Karlsruhe, Germany
Tim Pruessmann
Karlsruhe Institute of Technology (KIT), Institute for Nuclear Waste Disposal, P.O. Box 3640, 76021 Karlsruhe, Germany
Jörg Rothe
Karlsruhe Institute of Technology (KIT), Institute for Nuclear Waste Disposal, P.O. Box 3640, 76021 Karlsruhe, Germany
Dieter Schild
Karlsruhe Institute of Technology (KIT), Institute for Nuclear Waste Disposal, P.O. Box 3640, 76021 Karlsruhe, Germany
Arndt Walschburger
Karlsruhe Institute of Technology (KIT), Institute for Nuclear Waste Disposal, P.O. Box 3640, 76021 Karlsruhe, Germany
Horst Geckeis
Karlsruhe Institute of Technology (KIT), Institute for Nuclear Waste Disposal, P.O. Box 3640, 76021 Karlsruhe, Germany
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The present contribution provides an overview on the collaborative project iCROSS and reports selected results. The impact of considering complex coupled processes in repository subsystems for the assessment of the integrity of a given (generic) repository arrangement will be discussed. The interdisciplinary team combines experimental work in the lab, in the underground rock laboratory and environmental simulations in order to achieve process understanding across variable scales.
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An overview on the recent advances in the field of high temperature studies of radionuclides in aqueous solutions will be given. Besides summarizing information on key technical aspects relevant for high temperature studies, the effect of increased temperatures on the complexation of trivalent actinides with chloride will be discussed in more detail, to illustrate newly derived in-depth understanding of the impact of increased temperatures on the (geo)chemical behaviour of trivalent actinides.
Cited articles
ESK: Diskussionspapier zur verlängerten Zwischenlagerung bestrahlter Brennelemente und sonstiger Wärme entwickelnder radioaktiver Abfälle, Entsorgungskommission, Bonn, Deutschland, 2015.
Ewing, R. C.: Long-term storage of spent nuclear fuel, Nat. Mater., 14, 252–257, 2015.