Articles | Volume 1
https://doi.org/10.5194/sand-1-159-2021
https://doi.org/10.5194/sand-1-159-2021
Conference Abstract
 | 
10 Nov 2021
Conference Abstract |  | 10 Nov 2021

Impact of increased temperatures on the geochemical behaviour of trivalent actinides in aquatic systems

Andrej Skerencak-Frech, Petra Panak, Kathy Dardenne, Jörg Rothe, Xavier Gaona, Marcus Altmaier, and Horst Geckeis

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Cement as a component of the multi-barrier system: radionuclide retention in cementitious environments
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Saf. Nucl. Waste Disposal, 1, 151–152, https://doi.org/10.5194/sand-1-151-2021,https://doi.org/10.5194/sand-1-151-2021, 2021

Cited articles

Grenthe, I., Gaona, X., Plyasunov, A. V., Linfeng, R., Runde, W. H., Grambow, B., Konings, R. J., Smith, A. L., and Moore, E. E.: Second Update on the chemical Thermodynamics of Uranium, Neptunium, Plutonium, Americium and Technetium, vol 14, OECD Publications, Paris, France, 2020.  
Skerencak-Frech, A., Fröhlich, D. R., Rothe, J., Dardenne, K., and Panak, P. J.: Combined Time-Resolved Laser Fluorescence Spectroscopy and Extended X-ray Absorption Fine Structure Spectroscopy Study on the Complexation of Trivalent Actinides with Chloride at T=25–200 C, Inorg. Chem., 53, 1062–1069, https://doi.org/10.1021/ic4025603, 2014. 
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Short summary
An overview on the recent advances in the field of high temperature studies of radionuclides in aqueous solutions will be given. Besides summarizing information on key technical aspects relevant for high temperature studies, the effect of increased temperatures on the complexation of trivalent actinides with chloride will be discussed in more detail, to illustrate newly derived in-depth understanding of the impact of increased temperatures on the (geo)chemical behaviour of trivalent actinides.